Journal
CHEMICAL COMMUNICATIONS
Volume 58, Issue 56, Pages 7817-7820Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc02451a
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Funding
- National Natural Science Foundation of China [22073057]
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In this study, porous Ce-CoP nanosheets were designed through a deep eutectic solvent approach, and they achieved efficient electrooxidation of HMF to FDCA. In 1 M KOH electrolyte, the conversion of HMF, the yield of FDCA, and the faradaic efficiency were all at high levels.
The electrooxidation of 5-hydroxymethylfurfural (HMF) to 2,5-furanedioic acid (FDCA) has received increasing attention. To achieve satisfactory electrooxidation of HMF, the development of an efficient electrocatalyst is particularly critical. Herein, porous Ce-CoP nanosheets integrating Ce doping and P vacancies are designed through a deep eutectic solvent approach, and they allow the excellent electrocatalytic oxidation of HMF to FDCA in 1 M KOH electrolyte with 100% HMF conversion, 98% FDCA yield, and a faradaic efficiency of 96.4% at low potential.
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