4.6 Article

Structural phase transition and superconductivity of ytterbium under high pressure

Journal

PHYSICAL REVIEW B
Volume 105, Issue 21, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevB.105.214503

Keywords

-

Funding

  1. National Natural Science Foundation of China [12111530103, 12174352]
  2. CAEP Project [TCGH0710]

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The study on the structural phase transition and superconductivity of late lanthanide ytterbium (Yb) metal under high pressure revealed the serendipitous discovery of the P6(3)/mmc phase as a superior superconductor with a critical temperature higher than other known RE elemental superconductors.
Recent advances in theory and experiment declare the rare-earth (RE) hydrogen-rich compound LaH10 is a near room-temperature superconductor under high pressure. To understand the underlying mechanism of superconductivity and explore the crucial role of lanthanides in forming the RE-based polyhydrides, we here perform a theoretical study on the structural phase transition and superconductivity of late lanthanide ytterbium (Yb) metal under high pressure up to 240 GPa. Two alternative structures, R (3) over barm and I4/mmm phases, of Yb are presented. Most interestingly, the P6(3)/mmc phase of Yb is serendipitously discovered to be a superior superconductor with a critical temperature value of 19.5 K at 160 GPa, which is higher than other known RE elemental superconductors. The present findings establish an alternative structural phase transition sequence of Yb, which offers insights for further understanding the vital physics mechanisms of a lanthanide-based superconductor.

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