Tunable surface plasmon resonance enhanced fluorescence via the stretching of a gold quantum dot-coated aluminum-coated elastomeric grating substrate

In this study, the surface plasmon resonance (SPR)-enhanced fluorescence properties of gold quantum dots (AuQDs) on an aluminum (Al)-coated polydimethylsiloxane (PDMS) grating substrate were investigated by changing the grating pitch via mechanical stretching. The SPR-excitation wavelength of the AuQDs/Al-coated PDMS-grating substrate was tuned by changing the incident light angle from 5 degrees to 60 degrees and stretching it from 0 to 1.0 mm. In addition, the SPR-enhanced fluorescence tuning ability was studied using an AuQD/Al-coated PDMS-grating film by stretching the substrate. The SPR-enhanced fluorescence (SPF) of the AuQDs on the Al-grating was observed using a violet laser as the excitation source at 405 nm with p-polarization. The wavelengths of the SPR excitation, corresponding to the SP-dispersion mode of +1, were shifted to a longer wavelength upon stretching the grating substrate from 0 to 1.0 mm. By stretching the AuQDs/Al-grating PDMS substrate, the SPR-enhanced fluorescence intensity increased at fixed incident angles of 15 degrees and 35 degrees, whereas the SPR-enhanced fluorescence intensity decreased at 40 degrees. Moreover, the SPF could be tuned to exhibit different properties in tunable optical sensors.

Automated summary

In this study, the SPR-enhanced fluorescence properties of AuQDs on an Al-coated PDMS grating substrate were investigated by changing the grating pitch through mechanical stretching. The results showed that stretching the grating substrate can tune the SPR excitation wavelength and enhance the fluorescence intensity, which is promising for applications in tunable optical sensors.