Journal
CHEMICAL COMMUNICATIONS
Volume 58, Issue 81, Pages 11402-11405Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2cc03285f
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Funding
- Kyoto University's Overseas On-site Laboratory Program
- KAKENHI [JP22H05005]
- A*STAR Central Research Fund
- A*STAR Computational Resource Centre
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This study presents a direct method for synthesizing UiO-66 MOFs using adipic acid as a linker, which is traditionally overlooked. The research also demonstrates the feasibility of using adipic acid for MOF defect engineering.
Adipic acid, an industrially-important chemical that can be sustainably derived from biomass and post-consumer nylon, is traditionally overlooked as a linker for MOFs. Herein, we report the first direct one-pot method for synthesising UiO-66 MOFs with an unprecedented 69 mol% adipate content, as well as the feasibility of these materials for MOF defect engineering by rapid and selective adipate thermolysis.
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