Journal
CRYSTENGCOMM
Volume 24, Issue 43, Pages -Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d2ce01170k
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Funding
- DFG [SPP 1928, Ja466/43-1]
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The first use of a bulky barrel-shaped ligand in HHUD-3 is demonstrated, which shows accessible porosity only feasible for a defect structure. With 35%+ missing linker defects and S-BET = 890 m(2)g(-1) (N-2), HHUD-3 exhibits higher CH4 adsorption but lower CO2 and H-2 adsorption compared to UiO-66.
The first use of a bulky barrel-shaped ligand is demonstrated in HHUD-3, with accessible porosity only feasible for a defect structure. With 35%+ missing linker defects and S-BET = 890 m(2)g(-1) (N-2), HHUD-3 features higher CH4 but lower CO2 and H-2 adsorption than UiO-66.
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