Journal
NANO-MICRO LETTERS
Volume 8, Issue 4, Pages 381-387Publisher
SHANGHAI JIAO TONG UNIV PRESS
DOI: 10.1007/s40820-016-0099-z
Keywords
Zn-doped TiO2 nanotubes; ZnO nanoflakes; Heterostructures; DSSC
Funding
- UGC-DAE CSR, Indore
- Michigan Space Grant Consortium
- Hope College
- DAE-BRNS
- Division Of Physics
- Direct For Mathematical & Physical Scien [1613188] Funding Source: National Science Foundation
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The paper reports the fabrication of Zn-doped TiO2 nanotubes (Zn-TONT)/ZnO nanoflakes heterostructure for the first time, which shows improved performance as a photoanode in dye-sensitized solar cell (DSSC). The layered structure of this novel nanoporous structure has been analyzed unambiguously by Rutherford backscattering spectroscopy, scanning electron microscopy, and X-ray diffractometer. The cell using the heterostructure as photoanode manifests an enhancement of about an order in the magnitude of the short circuit current and a seven-fold increase in efficiency, over pure TiO2 photoanodes. Characterizations further reveal that the Zn-TONT is preferentially oriented in [001] direction and there is a Ti metal-depleted interface layer which leads to better band alignment in DSSC.
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