Journal
METALS
Volume 6, Issue 7, Pages -Publisher
MDPI
DOI: 10.3390/met6070147
Keywords
microstructure; photoconversion; solar cell; perovskite; Sb; Cl; NH4Cl; antimony
Funding
- Satellite Cluster Program of the Japan Science and Technology Agency [25420760]
- Grants-in-Aid for Scientific Research [25420760] Funding Source: KAKEN
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The effects of SbI3, PbCl2, and NH4Cl addition to perovskite CH3NH3PbI3 precursor solutions on photovoltaic properties were investigated. TiO2/CH3NH3Pb(Sb)I-3(Cl)-based photovoltaic devices were fabricated by a spin-coating technique, and the microstructures of the devices were investigated by X-ray diffraction and scanning electron microscopy. Current density-voltage characteristics and incident photon-to-current conversion efficiencies were improved by a small amount of Sb- and Cl-doping, which resulted in improvement of the efficiencies of the devices. The structure analysis indicated formation of a homogeneous microstructure by NH4Cl addition with SbI3.
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