Journal
CHINESE JOURNAL OF CATALYSIS
Volume 43, Issue 12, Pages 3019-3045Publisher
ELSEVIER
DOI: 10.1016/S1872-2067(22)64150-0
Keywords
Hydrogen production; Homogeneous catalysis; Earth abundant metal; Electrocatalysis; Ligand design
Funding
- National Science Foundation [CHE-1352036, CHE-2018806, CHE-2102265]
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This review article introduces the rational design of molecular metal complexes based on earth-abundant metals for electrocatalytic hydrogen production. It emphasizes providing insight into structure-function relationships in catalytic properties for future ligand and catalyst design.
For public health and environmental protection reasons, there is an urgent need to replace tradi-tional fossil fuels with clean and renewable sources. Electrochemical splitting of water has the po-tential to produce clean hydrogen as a possible solution to global energy problems. This review article introduces the rational design of molecular metal complexes based on earth-abundant met-als for electrocatalytic hydrogen production in water or water-organic media. Emphasis is placed on providing insight into structure-function relationships in catalytic properties for future ligand and catalyst design.(c) 2022, Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved.
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