4.6 Article

Electrodynamic Modeling of Quantum Dot Luminescence in Plasmonic Metamaterials

Journal

ACS PHOTONICS
Volume 3, Issue 4, Pages 558-563

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.5b00499

Keywords

photoluminescence; plasmonics; metamaterials; quantum dots; finite-different time-domain; spontaneous emission

Funding

  1. U.S. Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) [DE-AC02-07CH11358]
  2. National Natural Science Foundation of China [61101064, 51277001, 51477039, 61201122]
  3. NCET of China [NCET-12-0596]
  4. DFMEC [20123401110009]
  5. European Research Council under ERC Advanced Grant (PHOTOMETA) [320081]
  6. Anhui Provincial Natural Science Foundation [1508085JD03, 1508185QF130]
  7. European Research Council (ERC) [320081] Funding Source: European Research Council (ERC)

Ask authors/readers for more resources

A self-consistent approach is proposed to simulate a coupled system of quantum dots (QDs) and metallic metamaterials. Using a four-level atomic system, an artificial source is introduced to simulate the spontaneous emission process in the QDs. We numerically show that the metamaterials can lead to multifold enhancement and spectral narrowing of photoluminescence from QDs. These results are consistent with recent experimental studies. The proposed method represents an essential step for developing and understanding a metamaterial system with gain medium inclusions.

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