Journal
JOURNAL OF PHYSICAL CHEMISTRY C
Volume 126, Issue 37, Pages 15864-15872Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.jpcc.2c0559815864
Keywords
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Funding
- National Key R&D Program of China [2017YFA0304203]
- National Natural Science Foundation of China [62020106014, 62175140, 61901249, 92165106, 12104276]
- PCSIRT [IRT--17R70]
- 111 project [D18001]
- Program for the Outstanding Innovative Teams of Higher Learning Institutions of Shanxi (OIT)
- Applied Basic Research Project of Shanxi Province, China [201901D211191, 201901D211188]
- Shanxi 1331 KSC
- Russian Foundation for Basic Research
- NSF of China [62011530047, 20- 53-53025]
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A fluorescence-based evaporation sensor utilizing the photoluminescence property of monolayer MoS2 and the dielectric screening effect of micro-droplets is developed. This sensor can identify different liquids and monitor the evaporation process of micro-droplets.
Herein, an optical evaporation sensor is achieved based on the photoluminescence (PL) property of monolayer MoS2 through the micro-droplet dielectric screening effect. The emission intensity, full width at half-maximum, photon energy, and intensity ratio of two excitons are related to the dielectric constant of the micro-droplets, which are employed to recognize the kind of liquids. During the evaporation process of volatile organic compound micro-droplets, the collected PL intensity is significantly affected by the refractive index. The theoretical model of a micro-droplet evaporation sensor based on the dielectric screening effect is established and verified by the finite-difference time-domain and the finite-element method. This work processes a fluorescent probe technique for micro-droplet recognition and evaporation monitoring with non-contact, high precision, and miniaturization.
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