Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 4, Issue 19, Pages 7174-7177Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ta00431h
Keywords
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Funding
- 973 Program [2013CB834704, 2014CB932103]
- Provincial Key Project of China [7131253]
- National Natural Science Foundation of China [21231002, 21276026, 21201018, 21404010, 21471018]
- 1000 Plan (Youth)
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A copper(II)-based MOF film (MOF-199/Ni) prepared by electrodeposition shows exceptionally high photocatalytic hydrogen production rates of 8000 mmol h(-1) g(-1) (based on the mass of MOF-199) and 24 400 mmol h(-1) g(-1) with Pt as the co-catalyst and eosin Y as the photosensitizer. The activity is one of the highest among all the reported-MOF-based hydrogen production systems. With nickel foam as a substrate, the deactivation of MOF-199 is largely alleviated, and the MOF-199/Ni film can be easily recycled and reused after photocatalytic hydrogen production.
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