Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 4, Issue 15, Pages 5366-5384Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ta00265j
Keywords
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Funding
- Human Resource Training Program for Regional Innovation and Creativity through the Ministry of Education
- National Research Foundation of Korea [NRF-2014H1C1A1073093]
- National Research Foundation of Korea Grant - Ministry of Education [NRF-2014R1A1A2057691]
- Human Resources Development program of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant - Korea government Ministry of Trade, Industry and Energy [20124010203310]
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Silicon-based composites are very promising anode materials for boosting the energy density of lithium-ion batteries (LIBs). These silicon-based anodes can also replace the dendrite forming lithium metal anodes in lithium metal-free Li-O-2 and Li-S batteries, which can offer energy content far beyond that of current LIBs. However, it is challenging to design silicon-based materials for use as anodes in real energy storage devices. In this review, we discuss how to boost the energy content of LIBs, the pros and cons of silicon-based anodes, and challenges associated with silicon-based anodes. A major focus of this review is on the rational design of silicon-based composite anodes to address the outstanding issues. In addition, high energy LIBs and Li-S batteries that employ silicon-based anodes are introduced and discussed.
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