Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 4, Issue 36, Pages 14017-14024Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ta06657g
Keywords
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Funding
- Recruitment Program of Global Youth Experts
- National High-tech R&D Program of China (863 Program) [2015AA034601]
- National Natural Science Foundation of China [21474035, 51403071]
- Fundamental Research Funds for the Central Universities, HUST [2016JCTD111]
- Science and Technology Program of Shenzhen [JCYJ20160429182443609]
- China Postdoctoral Science Foundation [2015T80794]
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Flexible and light-weight photovoltaics are desirable for applications that involve their integration with flexible electronics. In this study, we demonstrate efficient flexible perovskite solar cells with a novel device architecture (that is indium-tin-oxide (ITO) free and top-illuminated) using a low-temperature processed doped fullerene as the electron-transporting layer. Silver is used as the bottom electrode, and a transparent conducting polymer electrode is used as the top electrode for light illuminating through to the active layer. Stearyldimethylbenzylammonium chloride (SDBAC)-doped [6,6]-phenyl-C-61-butyric acid methyl ester (PC61BM) was the electron-transporting layer wherein SDBAC could enhance the conductivity by three orders of magnitude and therefore enhance the solar cell performance. The ITO-free flexible perovskite solar cells display power conversion efficiency of 11.8% on a polyethersulfone substrate and can maintain 84% of the initial PCE after 1000 bending cycles at a bending radius of 6 mm.
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