Journal
CURRENT OPINION IN CHEMICAL ENGINEERING
Volume 42, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.coche.2023.100969
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This study examines the importance of energy management in catalyst design and catalysis process development, and explores the impact of temperature on solid-based catalysis. By analyzing innovative heating techniques and temperature-monitoring technologies, the study demonstrates the potential for transformative industrial catalytic processes.
To the achievement of carbon neutrality and sustainable chemical industries, optimization and reformation of energy (heat) management for catalyst design and catalysis process developments play a key role. This review examines the underlying mechanism of fundamental solid-based catalysis, for example, structure of active sites, chemical kinetics, and molecular transport, affected by temperature. In situ/operando multiscale thermometry aimed to the temperature-monitoring of local active sites, catalyst body, or reactor is overviewed. Toward precise heat supply for active sites, the examples of state-of-the-art heating techniques for solid catalysts are analyzed in detail. Through recent examples, we illustrate that innovative heating techniques combined with online spatiotemporal-resolved thermometry may initiate transformative industrial catalytic processes.
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