Journal
GREEN CHEMISTRY
Volume -, Issue -, Pages -Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d3gc03389a
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A solvent-tuned electrochemical protocol for the selective transfer hydrogenation of imidazopyridines using carbazates as hydrogen donors has been developed, providing a more sustainable and greener way to access partially saturated N-heterocycles by avoiding traditionally employed transition metal catalysts and high-pressure hydrogen. This method is scalable and applicable to late-stage functionalization of complex molecules.
A solvent-tuned electrochemical protocol for the selective transfer hydrogenation of imidazopyridines using carbazates as hydrogen donors has been developed. This electrosynthesis strategy provides a more sustainable and greener way to access partially saturated N-heterocycles by avoiding traditionally employed transition metal catalysts and high-pressure hydrogen. Remarkably, the method is scalable and applicable to late-stage functionalization of complex molecules. A possible mechanism has been proposed on the basis of radical-trapping and cyclic voltammetry experiments. A solvent-tuned electrochemical protocol for the selective transfer hydrogenation of imidazopyridines using carbazates as hydrogen donors has been developed.
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