Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 62, Issue 40, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202311352
Keywords
Fullerene; Hydrogen; Hydrogen Peroxide; Nanosheet; Solar Water Splitting
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This study demonstrates the interesting photocatalytic performance of few-layer fullerene network in pure water splitting, showing high evolution rates and stability.
A few-layer fullerene network possesses several advantageous characteristics, including a large surface area, abundant active sites, high charge mobility, and an appropriate band gap and band edge for solar water splitting. Herein, we report for the first time that the few-layer fullerene network shows interesting photocatalytic performance in pure water splitting into H-2 and H2O2 in the absence of any sacrificial reagents. Under optimal conditions, the H-2 and H2O2 evolution rates can reach 91 and 116 mu molg(-1)h(-1), respectively, with good stability. This work demonstrates the novel application of the few-layer fullerene network in the field of energy conversion.
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