Journal
MATERIALS CHEMISTRY FRONTIERS
Volume -, Issue -, Pages -Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d3qm00835e
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Metal-organic frameworks (MOFs)-derived materials, as competitive electrocatalysts, have great potential in the electrochemical reduction of CO2 into fuel/high-value chemicals using electricity generated from renewable energy. This review systematically summarizes various synthesis strategies to fabricate diverse and functional MOF-derived materials, and classifies their applications in detail according to the reduction products in the CO2 reduction reaction.
Electrochemical reduction of CO2 into fuel/high-value chemicals using electricity generated from renewable energy is one of the most promising ways to achieve carbon neutrality. Recently, metal-organic frameworks (MOFs)-derived materials, originating from the MOF architecture, show competitive performance as electrocatalysts in CO2 reduction. This review systematically summarizes several synthesis strategies to fabricate diverse and functional MOF-derived materials including pyrolysis, precursor regulation, post-modification and other synthesis. Additionally, the application of MOF-derived materials in the ECO2RR is classified in detail according to the reduction products. Eventually, some challenges and prospects of the synthesis of MOF-derived electrocatalysts and their application in ECO2RR are presented.
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