Journal
ASIAN JOURNAL OF ORGANIC CHEMISTRY
Volume 5, Issue 10, Pages 1204-1207Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ajoc.201600338
Keywords
C-H functionalization; heterocycles; redox; regioselectivity; tetrahydroisoquinoline
Categories
Funding
- National Program on Key Research Project [2016YFA0602900]
- National Natural Science Foundation of China [21472249]
- Natural Science Funds of Guangdong Province for Distinguished Young Scholar [2016A030306029]
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A silver or acid-mediated three-component reaction of tetrahydroisoquinolines, benzaldehydes, and diazo compounds has been developed. The reaction provides a novel route to beta-amino-alpha-diazo compounds through redox-neutral C1 functionalization of unprotected THIQs with diazo carbonyl motifs with high regioselectivity.
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