Journal
CHEMELECTROCHEM
Volume 10, Issue 19, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/celc.202300370
Keywords
electrocatalysis; spectroscopy; ethanol oxidation reaction; insitu Raman spectroscopy; reaction mechanism
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The Electrochemical Ethanol Oxidation Reaction (EOR) is crucial in energy conversion devices. In situ Raman spectroscopy is an invaluable tool for identifying intermediates and inferring the reaction mechanism, making it one of the most suitable methods for studying EOR.
The Electrochemical Ethanol Oxidation Reaction (EOR) plays a pivotal role in next-generation energy conversion devices. A clear understanding of the EOR reaction mechanism is critical for rational catalyst design, a task complicated by the numerous reaction intermediates and pathways involved. To this end, insitu Raman spectroscopy has proven invaluable in identifying many such intermediates at the electrode/electrolyte interface under varying applied potentials. Therefore, this technique allows for inference of the reaction mechanism based on the detected Raman signals of intermediates and observed structural changes, positioning insitu Raman spectroscopy as one of the most suitable methods for studying the EOR reaction mechanism. In this short review, with an eye towards future applications, we concentrate on the essential fundamentals of EOR and highlight recent advancements in understanding the EOR mechanism by insitu Raman spectroscopy.
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