Journal
ADVANCED OPTICAL MATERIALS
Volume 5, Issue 2, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adom.201600819
Keywords
fill factor; large area; organohalide perovskite solar cells; sheet resistance
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Funding
- International Postgraduate Research Scholarship (IPRS)
- Australian Research Council [DP 140102379]
- Australian Government through the Australian Renewable Energy Agency (ARENA) Australian Centre for Advanced Photovoltaics
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Thin film organohalide lead perovskite-based solar cells have emerged over the last five years as a potentially low-cost, low-embedded-energy and high-efficiency photovoltaic technology. However, almost all reported high-efficiency devices have small active areas significantly less than 1 cm(2). Upscaling of organohalide lead perovskite solar cells is now required for successful manufacturing and commercialization. In this work, three generic design rules for large area devices are proposed. Using these design rules, high efficiency large area (2.0 cm(2)) cells are demonstrated based on a predictive methodology incorporating the optoelectronic design of highly transparent and conductive electrodes, and controlled crystal size and uniformity of the organohalide perovskite junction. These optimized large area monolithic solar cells show power conversion efficiencies (PCEs) >12%, with an enhanced open-circuit voltage (V-oc) of 1.02 V and respectable fill factor (FF) of 0.61.
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