Journal
ENVIRONMENTAL SCIENCE & TECHNOLOGY
Volume 57, Issue 48, Pages 19565-19574Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.est.3c05050
Keywords
methane; greenhouse gas; urban; emissions
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This study reveals that urban methane emissions in Washington, DC, and Baltimore, Maryland exceed estimates derived from traditional inventory methods. The study shows a decreasing trend in annual emissions over a four-year period and identifies wintertime emissions to be 44% higher than summertime emissions, correlating with natural gas consumption. Spatially resolved estimates attribute a significant portion of methane emissions to the natural gas sector, supporting previous findings. This research contributes to our understanding of urban methane emissions and provides evidence for mitigating natural gas emissions.
Urban methane emissions estimated using atmospheric observations have been found to exceed estimates derived by using traditional inventory methods in several northeastern US cities. In this work, we leveraged a nearly five-year record of observations from a dense tower network coupled with a newly developed high-resolution emissions map to quantify methane emission rates in Washington, DC, and Baltimore, Maryland. Annual emissions averaged over 2018-2021 were 80.1 [95% CI: 61.2, 98.9] Gg in the Washington, DC urban area and 47.4 [95% CI: 35.9, 58.5] Gg in the Baltimore urban area, with a decreasing trend of approximately 4-5% per year in both cities. We also find wintertime emissions 44% higher than summertime emissions, correlating with natural gas consumption. We further attribute a large fraction of total methane emissions to the natural gas sector using a least-squares regression on our spatially resolved estimates, supporting previous findings that natural gas systems emit the plurality of methane in both cities. This study contributes to the relatively sparse existing knowledge base of urban methane emissions sources and variability, adding to our understanding of how these emissions change in time and providing evidence to support efforts to mitigate natural gas emissions.
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