Journal
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
Volume 26, Issue 2, Pages 1322-1327Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d3cp04962k
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The atomic structure of the Ag(111)-p(4 x 4)-O phase was reexamined and two phases with the same periodicity were discovered. It was demonstrated that the accepted Ag6 model is incompatible with high-resolution oxygen-sensitive STM images.
The atomic structure of the Ag(111)-p(4 x 4)-O phase was reexamined with scanning tunneling microscopy (STM) and density functional theory. We discovered two different phases with the same (4 x 4) periodicity and demonstrated that the accepted Ag6 model is incompatible with high-resolution oxygen-sensitive STM images. Using bias dependencies of the STM images, we have shown that the p(4 x 4) phase is highly nonuniform, with local oxygen coverage varying from 1/8 ML up to 1/2 ML.
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