4.7 Article

Satellite observations of smoke-cloud-radiation interactions over the Amazon rainforest

Journal

ATMOSPHERIC CHEMISTRY AND PHYSICS
Volume 23, Issue 7, Pages 4595-4616

Publisher

COPERNICUS GESELLSCHAFT MBH
DOI: 10.5194/acp-23-4595-2023

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This study investigates the smoke-cloud-radiation interactions in the Amazon rainforest using satellite sensors. The results show that smoke significantly modifies the Amazonian atmosphere and has different effects on convective activity, cloudiness, and precipitation depending on the smoke concentration. Further research is needed to understand the impact of smoke on the Amazon climate.
The Amazon rainforest routinely experiences intense and long-lived biomass burning events that result in smoke plumes that cover vast regions. The spatial and temporal extent of the plumes and the complex pathways through which they interact with the atmosphere have proved challenging to measure for purposes of gaining a representative understanding of smoke impacts on the Amazonian atmosphere. In this study, we use multiple collocated satellite sensors on board AQUA and TERRA platforms to study the underlying smoke-cloud-radiation interactions during the diurnal cycle. An 18-year time series for both morning and afternoon overpasses is constructed, providing collocated measurements of aerosol optical depth (AOD; column-integrated aerosol extinction), cloud properties, top-of-atmosphere radiative fluxes, precipitation, and column water vapour content from independent sources.The long-term time series reduces the impact of interannual variability and provides robust evidence that smoke significantly modifies the Amazonian atmosphere. Low loadings of smoke (AOD <= 0.4) enhance convective activity, cloudiness, and precipitation, but higher loadings (AOD > 0.4) strongly suppress afternoon convection and promote low-level cloud occurrence. Accumulated precipitation increases with convective activity but remains elevated under high smoke loadings, suggesting fewer but more intense convective cells. Contrasting morning and afternoon cloud responses to smoke are observed, in line with recent simulations. Observations of top-of-atmosphere radiative fluxes support the findings and show that the response of low-level cloud properties and cirrus coverage to smoke results in a pronounced and consistent increase in top-of-atmosphere outgoing radiation (cooling) of up to 50 W m-2 for an AOD perturbation of +1.0.The results demonstrate that smoke strongly modifies the atmosphere over the Amazon via widespread changes to the cloud field properties. Rapid adjustments work alongside instantaneous radiative effects to drive a stronger cooling effect from smoke than previously thought, whilst contrasting morning and afternoon responses of liquid and ice water paths highlight a potential method for constraining aerosol impacts on climate. Increased drought susceptibility, land use change, and deforestation will have important and widespread impacts on the region over the coming decades. Based on this analysis, we anticipate that further increases in anthropogenic fire activity will associated with an overall reduction in regional precipitation and a negative forcing (cooling) on the Earth's energy budget.

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