4.6 Article

Interface based field effect configuration and charge conduction mechanisms for manganite thin film heterostructures

Journal

NEW JOURNAL OF CHEMISTRY
Volume 47, Issue 28, Pages 13508-13527

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/d3nj02070c

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Control over the movements of free charge carriers across manganite interfaces is achieved through external stimuli that alter electronic phases. A LaMnO3/La0.7Ca0.3MnO3/LaAlO3 (LMO/LCMO/LAO) manganite-manganite structure was successfully fabricated using a cost-effective chemical solution deposition (CSD) method. The resistive nature of the LMO/LCMO interface was studied using a field effect configuration and the impact of external electric fields on resistivity was discussed in terms of free charge carrier movements. The behavior of spin fluctuations in manganite lattices was analyzed using the Zener double exchange (ZDE) polynomial law.
Control over the movements of free charge carriers across any manganite based interface can functionalize the device for spintronic applications. This can be achieved through external stimuli that alter various electronic phases of manganites having comparable energy levels. In the present communication, the LaMnO3/La0.7Ca0.3MnO3/LaAlO3 (LMO/LCMO/LAO) manganite-manganite structure was successfully fabricated using a cost effective chemical solution deposition (CSD) method. Field effect configuration was employed to understand the interface resistive nature of the LMO/LCMO interface for which externally applied interface electric fields have been applied across the same interface. The applied interface electric field considerably affects the LMO/LCMO interface resistivity which has been discussed in the context of free charge carrier movements across the same interface. The state of the spin fluctuations across manganite lattices has been recognized by fitting the resistivity behavior theoretically using the Zener double exchange (ZDE) polynomial law. Complex electroresistance (ER) and anisotropic magnetoresistance (AMR) behaviors have been discussed in detail for understanding the electrical nature of the LMO/LCMO interface under different applied stimuli.

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