Journal
CHEMICAL COMMUNICATIONS
Volume 59, Issue 63, Pages 9615-9617Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/d3cc02285d
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A three-dimensional metal-covalent organic framework (3D-MCOF) called 3D-CTU-MCOF, based on cyclic trinuclear units, was synthesized using organic tetrahedral linkers and copper-based cyclic trinuclear complexes. This novel type of 3D-MCOF with ctn topology demonstrates enhanced electrocatalytic capacity for CO2 reduction reaction compared to independent cyclic trinuclear units.
A three-dimensional metal-covalent organic framework (3D-MCOF) based on cyclic trinuclear units was synthesized using organic tetrahedral linkers and copper-based cyclic trinuclear complexes. The novel type of 3D-MCOF, named 3D-CTU-MCOF, with the ctn topology, is reported herein for the first time. Our study demonstrated enhanced electrocatalytic capacity for CO2 reduction reaction of 3D-CTU-MCOF compared to independent cyclic trinuclear units.
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