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CATALYSIS SCIENCE & TECHNOLOGY
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ROYAL SOC CHEMISTRY
DOI: 10.1039/d3cy00834g
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Co-N-C catalysts were prepared by pyrolysis at 250-400°C for efficient oxidation of mono-phenols. 2,3,6-Trimethylphenol could be easily oxidized into 2,3,5-trimethyl-1,4-benzoquinone with dioxygen. Catalytic activity was not observed in CoO, Co3O4, or metallic Co particles, indicating that active Co(ii) species with N/O coordination dispersed on disordered carbonaceous materials.
Co-N-C catalysts were fabricated for efficient oxidation of mono-phenols after undergoing pyrolysis at 250-400 & DEG;C. 2,3,6-Trimethylphenol could be facilely oxidized into 2,3,5-trimethyl-1,4-benzoquinone with dioxygen. CoO, Co3O4 or metallic Co particles were excluded as catalytic active species, and active Co(ii) species with N/O coordination were dispersed on disordered carbonaceous materials.
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