Journal
JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
Volume 11, Issue 5, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.jece.2023.110634
Keywords
Solar-powered water evaporation; Holocellulose; Superhydrophilic; Salt-resistant; Seawater desalination
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This study presents an excellent salt-resistant solar steam evaporator for long-term interfacial solar water desalination by decorating polypyrrole (PPy) on the surface of holocellulose (HC). The PPy-HC evaporator exhibited superior salt-resistance and stability during long-term cycling test in high salinity brine, providing an effective solution for the issue of salt accumulation in traditional evaporators.
Interfacial solar-powered water evaporation is a cost-effective and sustainable approach using solar energy for seawater desalination. Nevertheless, salt accumulation during solar desalination generally restricts the wide-spread application of solar vapor generation. Herein, taking merits of the excellent hydrophilicity and inherent porosity of holocellulose (HC), An excellent salt-resistant solar steam evaporator for long-term interfacial solar water desalination was fabricated by decorating polypyrrole (PPy) on the surface of HC. Due to the broadband light absorbance of PPy and the superhydrophilic HC substrate, the PPy-HC evaporator exhibited a high evap-oration rate of 1.45 kg m � 2 h-1 and conversion efficiency of 93.4 % in a 5 wt% NaCl solution under one sun illumination. Importantly, the evaporator presented superior salt-resistance and stability during long-term cycling test in high salinity brine. This work reveals the key role of superhydrophilicity and water trans-portation capability in high salt solution solar-driven desalination. Thus, this work provides an effective approach to address the issue of salt accumulation of the traditional evaporator, demonstrating its great potential for real-world solar-driven seawater desalination.
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