Journal
SCIENTIFIC REPORTS
Volume 6, Issue -, Pages -Publisher
NATURE RESEARCH
DOI: 10.1038/srep22620
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Funding
- FAME
- MARCO
- DARPA
- MURI ARO program [W911NF-11-1-0362]
- Louisiana Board of Regents through the Board of Regents Support Fund [LEQSF(2012-15)-RD-A-23]
- Louisiana Board of Regents through the LA EPSCoR [LEQSF-EPS(2014)-PFUND-378]
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Van der Waals materials, existing in a range of thicknesses from monolayer to bulk, allow for interplay between surface and bulk nonlinearities, which otherwise dominate only at atomically-thin or bulk extremes, respectively. Here, we observe an unexpected peak in intensity of the generated second harmonic signal versus the thickness of Indium Selenide crystals, in contrast to the quadratic increase expected from thin crystals. We explain this by interference effects between surface and bulk nonlinearities, which offer a new handle on engineering the nonlinear optical response of 2D materials and their heterostructures.
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