Journal
RSC ADVANCES
Volume 6, Issue 89, Pages 86744-86751Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ra19529f
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Funding
- National Natural Science Foundation of China [31170514, 31370557]
- Jiangsu Province Natural Science Foundation of China [BK20150875]
- Graduate Cultivation Innovative Project of Jiangsu Province
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
- Doctoral Program of Higher Education [20113204110011]
- Analysis & Test Center of Nanjing Forestry University
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Today, flexible energy storage systems have become attractive alternatives for applications in portable electronic devices. This account reports a simple and low-cost dipping and polymerization method for preparing flexible and free-standing supercapacitor film electrodes. The process consisted of depositing polypyrrole (PPy) coating on the surface and inside the network of an entangled cellulose nanofibers (CNFs)/multi-walled carbon nanotubes (MWCNTs) film. The electrochemical performance of the resulting CNFs/MWCNTs/PPy hybrid electrode was evaluated and compared with that of CNFs/MWCNTs film electrodes. The CNFs/MWCNTs/PPy nanocomposite electrode exhibited a particular entangled 3D network structure with an elevated specific capacitance of 288 F g(-1), obtained at a scan rate of 5 mV s(-1). This value is higher than that of the CNFs/MWCNTs electrode, calculated to be 32.2 F g(-1). Furthermore, the CNFs/MWCNTs/PPy electrode exhibited excellent redox reversibility and cycle stability. This novel procedure could provide an effective method for achieving flexible, free-standing, high-performance, low-cost, and environmentally friendly materials for use in supercapacitor electrodes.
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