Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 6, Issue 8, Pages 2560-2564Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cy02072g
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Funding
- EPSRC [EP/K036548/1, EP/K014706/1]
- Royal Society
- European Union [604307]
- EPSRC [EP/K036548/2] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K036548/1, EP/K036548/2, EP/K014706/1] Funding Source: researchfish
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Mesopore incorporation into ZSM-5 enhances the dispersion of Pd nanoparticles throughout the hierarchical framework, significantly accelerating m-cresol conversion relative to a conventional microporous ZSM-5, and dramatically increasing selectivity towards the desired methylcyclohexane deoxygenated product. Increasing the acid site density further promotes m-cresol conversion and methylcyclohexane selectivity through efficient dehydration of the intermediate methylcyclohexanol.
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