Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 6, Issue 15, Pages 6152-6158Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cy00362a
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Funding
- University Grant Commissions (UGC-JRF) of India
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A highly porous, crystalline catechol porphyrin COF was synthesized and applied as an organocatalyst for the chemical fixation of carbon dioxide to synthesize value-added chemicals such as cyclic carbonates and oxazolidinones under solvent-free and transition-metal-free conditions. The high surface area and the functionalities of the COF catalyst act synergistically to activate the starting material. The 2,3-DhaTph shows excellent activity towards cyclic carbonates at the atmospheric pressure of carbon dioxide. Additionally, this catalytic system is recyclable in nature and provides a higher turnover number than previously reported organocatalysts.
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