Journal
ACS CATALYSIS
Volume 6, Issue 5, Pages 2965-2981Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.6b00428
Keywords
methane activation; methane valorization; heterogeneous catalysis; reaction mechanism; radical rebound mechanism; C-H bond activation; alkane functionalization
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Funding
- Dutch Science Foundation (NWO) through VIDI personal grant MetMOFCat
- Netherlands Center for Multiscale Catalytic Energy Conversion (MCEC), an NWO Gravitation programme - Ministry of Education, Culture and Science of the government of the Netherlands
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In this Perspective, we highlight the main challenges to be addressed in the development of heterogeneous catalysts for the direct functionalization of methane. Along with our personal view on current developments in this field, we outline the main mechanistic, engineering, and catalyst design issues that have hampered implementation of new technologies and highlight possible paths to overcome these problems.
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