Journal
ACS CATALYSIS
Volume 7, Issue 2, Pages 920-935Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.6b02585
Keywords
hydroxyapatite; macroligand; green sustainable chemistry; selective oxidation; selective reduction; one-pot reaction
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Green sustainable chemistry, achievable via careful catalyst design, minimizes waste generation and energy/material consumption, reducing risks, hazards, and costs. Apatites exhibit unique characteristics and are utilized to design high-performance heterogeneous metal catalysts featuring both monomeric surface metal complexes and metal nanoparticles on the apatite surface as macroligands. This approach, relying on well-defined active metal species on the apatite surface, corresponds to the bone-supported catalyst design concept and produces high-performance catalysts for liquid-phase organic syntheses: e.g., selective oxidations, hydrogenations/hydrogenolysis, carbon carbon bond formations, and CO2 fixation.
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