Journal
CHEMICAL SCIENCE
Volume 7, Issue 9, Pages 5798-5804Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6sc00513f
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Funding
- NSF [DMR-1453083, CHE08-40523, CHE09-46690]
- U. S. DOE Office of Science Facility at Brookhaven National Laboratory [DE-SC0012704]
- NSF CRIF:MU award [CHE04-43580]
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1602240] Funding Source: National Science Foundation
- Division Of Materials Research
- Direct For Mathematical & Physical Scien [1453083] Funding Source: National Science Foundation
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A novel Pt-bisacetylide small molecule (Pt-SM) featuring roller-wheel geometry was synthesized and characterized. When compared with conventional Pt-containing polymers and small molecules having dumbbell shaped structures, Pt-SM displays enhanced crystallinity and intermolecular pi-pi interactions, as well as favorable panchromatic absorption behaviors. Organic solar cells (OSCs) employing Pt-SM achieve power conversion efficiencies (PCEs) up to 5.9%, the highest reported so far for Pt-containing polymers and small molecules.
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