Journal
CHEMSUSCHEM
Volume 8, Issue 4, Pages 600-602Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201403338
Keywords
charging potential; energy storage; homogeneous catalysis; Li-O-2 batteries; redox mediators
Funding
- National Key Basic Research Program of China [2014CB932302, 2014CB932303]
- National Natural Science Foundation of China [21373111, 21403107]
- Natural Science Foundation of Jiangsu Province of Peoples R. China [BK2012309]
- Specialized Research Fund for the Doctoral Program of Higher Education of Peoples R. China [20120091120022]
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We show that by using a suitable soluble redox mediator, the charging overpotential can be reduced and the round-trip efficiency can be improved in an aprotic Li-O-2 battery. Not only do we explore a new redox couple, 10-methyl-10H-phenothiazine, as a soluble catalyst that improves the electrochemical performance, but we also propose possible challenges that need to be overcome for the future improvement of aprotic Li-O-2 batteries.
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