Journal
CHEMSUSCHEM
Volume 8, Issue 11, Pages 1845-1849Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cssc.201500103
Keywords
carbon dioxide; carbonates; epoxides; fluor; organocatalysis
Funding
- Region Wallonne in the frame of the CO2Green, Sinopliss, and Flycoat projects
- Belgian Science Policy in the frame of the Interuniversity Attraction Poles Programme-Functional Supramolecular Systems [IAP VII/5]
- Fonds National pour la Recherche Scientifique (F.R.S.-FNRS)
- University of Bordeaux
- University of LIEGE
- Conseil Regional d'Aquitaine
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The addition of fluorinated alcohols to onium salts provides highly efficient organocatalysts for the chemical fixation of CO2 into epoxides under mild experimental conditions. The combination of online kinetic studies, NMR titrations and DFT calculations allows understanding this synergistic effect that provides an active organocatalyst for CO2/epoxides coupling.
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