Journal
PHYSICAL REVIEW LETTERS
Volume 116, Issue 13, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.116.133001
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Funding
- Alexander von Humboldt Foundation
- NSERC discovery grant [RPGIN/419092-2013]
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We use differential holography to overcome the forward scattering problem in strong-field photoelectron holography. Our differential holograms of H-2 and D-2 molecules exhibit a fishbonelike structure, which arises from the backscattered part of the recolliding photoelectron wave packet. We demonstrate that the backscattering hologram can resolve the different nuclear dynamics between H-2 and D-2 with subangstrom spatial and subcycle temporal resolution. In addition, we show that attosecond electron dynamics can be resolved. These results open a new avenue for ultrafast studies of molecular dynamics in small molecules.
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