4.6 Article

MoS2 Nanosheets Supported on 3D Graphene Aerogel as a Highly Efficient Catalyst for Hydrogen Evolution

Journal

CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 45, Pages 15908-+

Publisher

WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201501964

Keywords

electrocatalysis; graphene; hydrogen evolution; molybdenum; nanosheets

Funding

  1. Australian Research Council (ARC) Future Fellowship project [FT110100800]
  2. DECRA project [DE140100619]
  3. Ministry of Science and Technology [2012DFR40240]
  4. China Scholarship Council [201306030039]
  5. UTS Chancellor's Postdoctoral Fellowship (CPDF)

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The development of efficient catalysts for electrochemical hydrogen evolution is essential for energy conversion technologies. Molybdenum disulfide (MoS2) has emerged as a promising electrocatalyst for hydrogen evolution reaction, and its performance greatly depends on its exposed edge sites and conductivity. Layered MoS2 nanosheets supported on a 3D graphene aerogel network (GA-MoS2) exhibit significant catalytic activity in hydrogen evolution. The GA-MoS2 composite displays a unique 3D architecture with large active surface areas, leading to high catalytic performance with low overpotential, high current density, and good stability.

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