Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 46, Pages 16318-16343Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201501735
Keywords
alkaloids; communesin; perophoramidine; total synthesis; vicinal quaternary stereocenters
Categories
Funding
- NSF [CHE-1145236]
- NIH [GM 033049]
- John Stauffer Memorial Fellowship
- Stanford Graduate Fellowship
- Direct For Mathematical & Physical Scien
- Division Of Chemistry [1360634] Funding Source: National Science Foundation
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The communesin alkaloids are a diverse family of Penicillium-derived alkaloids. Their caged-polycyclic structure and intriguing biological profiles have made these natural products attractive targets for total synthesis. Similarly, the ascidian-derived alkaloid, perophoramidine, is structurally related to the communesins and has also become a popular target for total synthesis. This review serves to summarize the many elegant approaches that have been developed to access the communesin alkaloids and perophoramidine. Likewise, strategies to access the communesin ring system are reviewed.
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