Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 41, Pages 14314-14318Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201502689
Keywords
amines; carbamates; carbon dioxide; diaryliodonium salts; three-component coupling
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Funding
- National Natural Science Foundation of China [21172078]
- National Basic Research Program of China (973 Program) [2011CB808600]
- Guangdong Natural Science Foundation [10351064101000000]
- Fundamental Research Funds for the Central Universities [2015zz038]
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A phosgene- and metal-free synthesis of O-aryl carbamates is realized through a three-component coupling of carbon dioxide, amines and diaryliodonium salts. The reaction only requires a base as the promoter, providing access to a diverse array of O-aryl carbamates in moderate to high yields with excellent chemoselectivity.
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