Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 33, Pages 11687-11691Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201502407
Keywords
enamine; hydrogen bonding acceptor; kinetics; organocatalysis
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Funding
- National Science Foundation [CHE-1401700]
- National Science Foundation of China [NSFC-21472018]
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A hydrogen bond acceptor plays an important role in the catalytic cycle of organo-enamine catalysis. It can effectively influence the rate of reaction through hydrogen bonding interaction with enammonium (N-protonated enamine intermediate). Our findings are supported by both kinetic experiments and quantum chemical calculations.
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