Journal
ORGANIC LETTERS
Volume 19, Issue 1, Pages 102-105Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b03378
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Funding
- MOST (973 project) [2015CB856600]
- NSFC [21502183]
- Chinese Academy of Science [XDB20020000]
- Fundamental Research Funds for the Central Universities [WK2060190041]
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An enantioselective carbohyl allylation of aldehydes with simple alkenes has been achieved via a one-pot protocol. consisting of a Pd-catalyzed allyic C-H borylation with. bis(pinanediolato)diboron and a chiral Bronsted acid catalyzed asymmetric allylborylation, delivering homoallylic alcohols in High yield's and with excellent diastereo- and enantioseledivities. The double chiral induction of chiral allylic borate and chiral phosphoric acid allows the reaction to give excellent. stereoselectivities.
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