Journal
ORGANIC LETTERS
Volume 18, Issue 3, Pages 452-455Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03497
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Funding
- National Natural Science Foundation of China (NSFC) [21372118]
- Foundation Research Project of Jiangsu Province (The Natural Science Foundation) [BK20141359]
- 333 High Level Talent Project of JiangSu Province
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Visible light along with 5 mol % eosin B catalyzed the first direct C-H phosphorylation of thiazole derivatives with diarylphosphine oxides by a photoredox process in the absence of an external oxidant. The scope of thiazoles and phosphine oxides was further investigated, as was functional group tolerance. The general and operational simplicity provides a novel metal and oxidant-free alternative for the formation of heteroaryl-P bonds, and only molecular hydrogen is generated as a byproduct.
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