Journal
ORGANIC LETTERS
Volume 18, Issue 18, Pages 4614-4617Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b02253
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Funding
- Natural Science Foundation of China [21572118, JQ201505]
- Natural Science Foundation of Shandong province [21572118, JQ201505]
- fundamental research and subject construction funds [2014JC008, 104.205.2.5]
- Zhong-Ying scholar award of Shandong University
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A novel early and late transition-metal relay catalysis has been developed by combining a gold-catalyzed Cydoisomerization and a Yb(OTf)(3)-catalyzed diastereoselective [3 + 2] cycloaddition with aziridines in a selective C-C bond cleavage mode. Various biologically significant complex nitrogen-containing spiro heterocycles were rapidly constructed from readily available starting materials under mild conditions.
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