Journal
ORGANIC LETTERS
Volume 18, Issue 3, Pages 520-523Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03551
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Funding
- National Natural Science Foundation of China [21225208, 21472137, 21532008]
- National Basic Research Program of China (973 Program) [2014CB745100]
- Tianjin Municipal Science & Technology Commission [14JCQNJC06200]
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A novel one-pot sequential transformation via decarboxylative Mannich reaction (DMR) and oxidative C-H amination of cyclic imines with beta-ketoacids is described. This methodology has been utilized to provide access to fused aziridines with excellent diastereoselectivity. Several examples of catalytic enantioselective sequential transformation are presented.
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