Journal
ORGANIC LETTERS
Volume 18, Issue 6, Pages 1306-1309Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b00227
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Funding
- NSFC [21272231, 21472186, 21525208]
- Dalian Institute of Chemical Physics, Chinese Academy of Sciences
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C-H activation of arenes has been established as an important strategy for heterocycle synthesis via annulations between arenes and unsaturated coupling partners. However, nitriles failed to act as such a coupling partner. Dioxazolones have been employed as a synthon of nitriles, and subsequent coupling with arenes such as N-sulfinylimines and benzimidates bearing a functionalizable directing group provided facile access to two classes of quinazolines under Co(III)-catalysis.
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