Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 11, Pages 4229-4232Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201406522
Keywords
C-C coupling; electron transfer; EPR spectroscopy; molybdenum; radical cations
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Funding
- Center of Innovative and Emerging Materials (CINEMA)
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Experimental (EPR) and theoretical (DFT) evidence is provided for radical cation formation as initial step in the Mo2Cl10-mediated dehydrogenative arene coupling. The initial electron transfer from methoxyarenes to molybdenum proceeds via an inner sphere mechanism.
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