Journal
OPTICS LETTERS
Volume 41, Issue 24, Pages 5793-5796Publisher
OPTICAL SOC AMER
DOI: 10.1364/OL.41.005793
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Funding
- Ministry of Education, Culture, Sports, Science, and Technology (MEXT)/Japan Society for the Promotion of Science (JSPS) KAKENHI [JP15H03704, JP15KK0164, JP16H01054, JP16H02214]
- Army Research Office (ARO) [W911NF-16-1-0339]
- Grants-in-Aid for Scientific Research [16H02214, 15K21727, 16H01054, 15KK0164] Funding Source: KAKEN
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We report the first observation of nonlinear harmonic generation and sum frequency generation (SFG) coupled with stimulated Raman scattering (SRS) via the second-order (chi((2))) and the third-order (chi((2))) nonlinearities in a silica microbottle resonator. The visible light emission due to third-harmonic generation (THG) was observed in both the output of a tapered fiber and the optical microscope images, which can be used to identify the axial mode profiles. SFG enabled by three-and four-wave mixing processes between the pump light and the light generated via SRS was also observed. Second-harmonic generation (SHG) and the SFG are enabled by. chi((2)) induced in silica by surface effects and multipole excitations. (C) 2016 Optical Society of America.
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