Journal
CHEMISTRY-A EUROPEAN JOURNAL
Volume 21, Issue 17, Pages 6547-6556Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.201500203
Keywords
aromaticity; electronic structure; energy conversion; phosphorus heterocycles; pi interactions
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Funding
- Ministere de la Recherche et de l'Enseignement Superieur
- CNRS
- Region Bretagne, China-French associated international laboratory in Functional Organophosphorus Materials, Balaton PHC [(830386K) - FR_12_TET_A044DF3B]
- French National Research Agency (ANR)/Research Grants Council (RGC) Joint Research Scheme (ANR MOLMAT)
- COST [CM10302]
- Hungarian Scientific Fund OTKA K [105417]
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We describe the synthesis and the physical properties of polyaromatic hydrocarbons (PAHs) containing a phosphorus atom at the edge. In particular, the impact of the successive addition of aromatic rings on the electronic properties was investigated by experimental (UV/Vis absorption, fluorescence, cyclic voltammetry) and theoretical studies (DFT). The physical properties recorded in solution and in the solid state showed that the P-containing PAHs exhibit properties expected for an emitter in white organic light-emitting diodes (WOLEDs).
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