Journal
CHEMISTRY OF MATERIALS
Volume 27, Issue 23, Pages 7903-7909Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.chemmater.5b02847
Keywords
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Funding
- National Research Foundation of Korea (NRF) grant - Korean Government (MEST) [2008-0061983]
- KOREA RESEARCH INSTITUTE of CHEMICAL TECHNOLOGY(KRICT)
- [KK1501-B00]
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Functional bio-MOF hollow spheres with controlled size in the 35-2000 mu m range were successfully synthesized by interfacial reaction using a continuous-flow droplet microfluidic system in a single step and one-flow strategy. The architecture of MIL-88A frameworks was extended from single-shell to double-shell hollow spheres. Moreover, various functional nanopartides (silica, cobalt, and UiO-66(Zr) MOF) were directly encapsulated in the single-shell hollow spheres, while maintaining the functionality of the cargo. In particular, three kinds of enzymes (glycerol dehydrogenase, horseradish peroxidase, and acetylcholinesterase) were also encapsulated inside the single-shell hollow spheres under mild conditions. The catalytic activity and the superior recyclability of the encapsulated enzymes were demonstrated against free enzymes.
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